Actually, in this circuit, the current \$I\$ is independent of the resistance \$R\$.
To see this, remove \$R\$ from the circuit and calculate \$I\$:
$$I = \frac{20V + 40V}{100\Omega + 200 \Omega} = 200\mathrm{mA}$$
Interestingly, this implies that the voltage between the nodes where \$R\$ was connected is:
$$20V - 200\mathrm{mA} \cdot 100 \Omega = 0V$$
This means that we can add \$R\$ back to the circuit and the solution doesn't change since there is no voltage between those nodes.
Thus, there is no value of \$R \ge 0\$ that will yield a current \$I = 80\mathrm{mA}\$.
However, if we allow \$R < 0\$, we have the interesting possibility of an infinity of solutions!
Writing a KCL equation at the top of \$R\$ yields
$$\frac{V_R}{R||100\Omega||200\Omega} = 0A$$
For \$R\ge 0\$, the only solution is \$V_R = 0\$ as derived above.
But, if we allow
$$R = - (100\Omega||200\Omega) = -66.67 \Omega$$
the denominator is infinite and thus, there is a solution for any \$V_R\$ and associated \$I\$!
This shouldn't actually be too surprising. The Thevenin equivalent circuit 'seen' by the resistor \$R\$ is given by
\$V_t = 0V\$
and
\$R_t = 100||200 \Omega = 66.67 \Omega\$
If we then parallel this equivalent circuit with an \$R = -66.67 \Omega\$ resistor, the new Thevenin equivalent becomes an open circuit.
This means that we can place a voltage source across \$R\$ and the voltage source will not supply any current.
In other words, we can temporarily place a voltage source across \$R\$ and, since the source supplies no current, remove the source and the voltage across \$R\$ will not change - the circuit will maintain that voltage across \$R\$.
Of course, there are no physical negative resistors (though we can approximate them with active circuits) so this is mostly academic.